Page 21 - 《华中农业大学学报（自然科学版）》2020年第5期

第 ５ 期 尚欢 等: SO ２ 在矿质颗粒物表面非均相反应研究进展 １ ５

chemistr y from２０１４to２０１６inwinterinBei j in g : insi g htsfrom [ １８ ] LIUC , MA Q X , LIU YC , etal．S y ner g isticreactionbetween
hi g hＧresolutionaerosolmasss p ectrometr y [ J ] ．Journalof g eoＧ SO ２andNO ２onmineraloxides : a p otentialformationp athwa y
p h y sicalresearchＧatmos p heres , ２０１９ , １２４ ( ２ ): １１３２Ｇ１１４７． ofsulfateaerosol [ J ] ．Ph y sicalchemistr ychemicalp h y sics ,
[ ６ ] LIW J , SHAO L Y , ZHANG DZ , etal．Areviewofsin g le ２０１２ , １４ ( ５ ): １６６８Ｇ１６７６．
aerosolp articlestudiesintheatmos p hereofEastAsia : morＧ [ １９ ] TOLEDANODS , HENRICH VE．KineticsofSO ２adsor p tion
p holo gy , mixin gstate , source , andhetero g eneousreactions [ J ] ． onp hotoexcitedαＧFe ２O ３ [ J ] ．The j ournalofp h y sicalchemisＧ
Journalofcleaner p roduction , ２０１６ , １１２ ( ２ ): １３３０Ｇ１３４９． tr yB , ２００１ , １０５ ( １８ ): ３８７２Ｇ３８７７．
[ ７ ] SULLIVAN RC , GUAZZOTTISA , SODEMAN D A , etal． [ ２０ ] LIKJ , KONGLD , ZHANZAKOVA A , etal．Hetero g eneous
Directobservationsoftheatmos p hericp rocessin g of Asian conversionofSO ２onnanoαＧFe ２O ３ : theeffectofmor p holo gy ,
mineraldust [ J ] ．Atmos p hericchemistr y & p h y sics , ２００７ , ７ li g htilluminationandrelativehumidit y [ J ] ．EnvironmentalsciＧ
( ５ ): １２１３Ｇ１２３６． ence : nano , ２０１９ , ６ ( ６ ): １８３８Ｇ１８５１．
[ ８ ] RAVISHANKARA AR．Hetero g eneousandmulti p hasechemistr y [ ２１ ] FU HB , WANGX , WU HB , etal．Hetero g eneousu p takeand
inthetro p os p here [ J ] ．Science , １９９７ , ２７６ ( ５３１５ ): １０５８Ｇ１０６５． oxidationofSO ２ onironoxides [ J ] ．Thej ournalofp h y sical
[ ９ ] ZHANGRY , WANGG H , GUOS , etal．Formationofurban chemistr yC , ２００７ , １１１ ( １６ ): ６０７７Ｇ６０８５．
finep articulatematter [ J ] ．Chemicalreviews , ２０１５ , １１５ ( １０ ): [ ２２ ]崔虎雄, 成天涛, 陈建民, 等 ．SO ２ 在 Fe ２O ３ 颗粒表面不同温度
３８０３Ｇ３８５５． 下非均相反应的实验模拟[ J ] ． 物理化学学报, ２００８ , ２４ ( １２ ):
[ １０ ] DENTENERFJ , CARMICHAELGR , ZHANGY , etal．Role ２３３１Ｇ２３３６．CUIHX , CHENGTT , CHENJM , etal．AsimuＧ
ofmineralaerosolasareactivesurfaceintheg lobaltro p oＧ latedhetero g eneousreactionofSO ２onthesurfaceofhematite
s p here [ J ] ．Journalof g eo p h y sicalresearchＧatmos p heres , １９９６ , atdifferenttem p eratures [ J ] ．Acta p h y sicoＧchimicasinica ,
１０１ ( D１７ ): ２２８６９Ｇ２２８８９． ２００８ , ２４ ( １２ ): ２３３１Ｇ２３３６ ( inChinesewithEn g lishabstract ) ．
[ １１ ] CHEN H , NANAYAKKARA CE , GRASSIAN V H．TitaniＧ [ ２３ ] YANG W W , MA QX , LIU YC , etal．Theeffectofwateron
um dioxide p hotocatal y sis in atmos p heric chemistr y [ J ] ． thehetero g eneousreactionsofSO ２andNH ３onthesurfacesof
Chemicalreviews , ２０１２ , １１２ ( １１ ): ５９１９Ｇ５９４８． αＧFe ２O ３andγＧAl ２O ３ [ J ] ．Environmentalscience : nano , ２０１９ ,
[ １２ ] USHERCR , ALＧHOSNEY H , CARLOSＧCUELLARS , etal． ６ ( ９ ): ２７４９Ｇ２７５８．
Alaborator ystud yofthehetero g eneousu p takeandoxidation [ ２４ ] WU L Y , TONGSR , ZHOU L , etal．S y ner g isticeffectsbeＧ
ofsulfurdioxideonmineraldustp articles [ J / OL ] ．Journalof tweenSO ２andHCOOHonαＧFe ２O ３ [ J ] ．The j ournalof p h y siＧ
g eo p h y sicalresearch , ２００２ , １０７ ( D２３ ): ４７１３ [ ２０２０Ｇ０４Ｇ２９ ] ．htＧ calchemistr yA , ２０１３ , １１７ ( １９ ): ３９７２Ｇ３９７９．
t p s :// doi．or g / １０．１０２９ / ２００２JD００２０５１ , ２００２． [ ２５ ] ZHAO X , KONG L D , SUN Z Y , etal．TheinteractionsbeＧ
[ １３ ] RUBASINGHEGEG , ELZEYS , BALTRUSAITISJ , etal．ReＧ tweenhetero g eneousu p takeandadsor p tionofsulfurdioxide
actionsonatmos p hericdustp articles : surfacep hotochemistr y andacetaldeh y deon hematite [ J ] ．Thej ournalofp h y sical
andsizeＧde p endentnanoscaleredoxchemistr y [ J ] ．Journalof chemistr yA , ２０１５ , １１９ ( １７ ): ４００１Ｇ４００８．
p h y sicalchemistr y letters , ２０１０ , １ ( １１ ): １７２９Ｇ１７３７． [ ２６ ] ZHANGX Y , ZHUANG GS , CHENJM , etal．Hetero g eneＧ
[ １４ ]王铃, 马庆鑫, 贺泓 ． 光照对 SO ２ 在矿质氧化物表面非均相反应 ousreactionsofsulfurdioxideont yp icalmineral p articles [ J ] ．
的影响[ J ] ． 环 境 科 学 学 报, ２０１８ , ３８ ( ３ ): １１５５Ｇ１１６２．WANG Thej ournalofp h y sicalchemistr yB , ２００６ , １１０ ( ２５ ): １２５８８Ｇ
L , MA QX , HE H．EffectofUVli g htonthehetero g eneous １２５９６．
reactionofSO ２ ondifferentmineraloxidesurfaces [ J ] ．Acta [ ２７ ] ULLERSTAM M , JOHNSON M S , VOGT R , etal．DRIFTS
scientiaecircumstantiae , ２０１８ , ３８ ( ３ ): １１５５Ｇ１１６２ ( in Chinese andKnudsencellstud yofthehetero g eneousreactivit yofSO ２
withEn g lishabstract ) ． andNO ２ on mineraldust [ J ] ．Atmos p hericchemistr y and
[ １５ ] SHANGJ , LIJ , ZHU T．Hetero g eneousreactionofSO ２on p h y sics , ２００３ , ３ ( ６ ): ２０４３Ｇ２０５１．
TiO ２p articles [ J ] ．ScienceChinachemistr y , ２０１０ , ５３ ( １２ ): [ ２８ ] MA QX , LIU YC , HEH．S y ner g isticeffectbetweenNO ２and
２６３７Ｇ２６４３． SO ２ intheiradsor p tionandreactiononγＧalumina [ J ] ．The j ourＧ
[ １６ ] MAQX , WANGL , CHUBW , etal．Contrar y roleofH ２Oand nalof p h y sicalchemistr yA , ２００８ , １１２ ( ２９ ): ６６３０Ｇ６６３５．
O ２inthekineticsofhetero g eneous p hotochemicalreactionsof [ ２９ ] MA Q X , WANG T , LIU C , etal．SO ２initiatestheefficient
SO ２onTiO ２ [ J ] ．The j ournalofp h y sicalchemistr yA , ２０１９ , conversionofNO ２toHONOonM g Osurface [ J ] ．EnvironmenＧ
１２３ ( ７ ): １３１１Ｇ１３１８． talscience&technolo gy , ２０１７ , ５１ ( ７ ): ３７６７Ｇ３７７５．
[ １７ ] NANAYAKKARACE , PETTIBONEABJ , GRASSIAN V H． [ ３０ ] WANG H H , ZHONG C , MA Q X , etal．Theadsor p tionand
Sulfurdioxideadsor p tionandp hotooxidationonisoto p icall y Ｇ oxidationofSO ２onM g Osurface : ex p erimentalandDFTcalcuＧ
labeledtitaniumdioxidenano p articlesurfaces : rolesofsurface lationstudies [ J ] ．Environmentalscience : nano , ２０２０ , ７ ( ４ ):
h y drox y l g rou p sandadsorbedwaterintheformationandstaＧ １０９２Ｇ１１０１．
bilit yofadsorbedsulfiteandsulfate [ J ] ．Ph y sicalchemistr y [ ３１ ] PARKJY , JANG M．Hetero g eneousp hotooxidationofsulfur
chemical p h y sics , ２０１２ , １４ ( １９ ): ６９５７Ｇ６９６６． dioxideinthep resenceofairborne mineraldustp articles [ J ] ．